Hi Spswytch,
You had your numbers in quotes. That was one problem. Another might have been you were only checking the first 5 rows. See if this works for you.
Sub ProcessAllWorksheets()
Dim wk As Worksheet
Dim Target As Range
For Each wk In ActiveWorkbook.Worksheets
wk.Select
For Each Target In Range("A1:A524")
Select Case Target.Value
Case 21
Range("B" & Target.Row).Value = "FTP Service Port"
Case 22
Range("B" & Target.Row).Value = "SSH Management Port"
Case 123
Range("B" & Target.Row).Value = "Network Time Protocol"
Case 2207
Range("B" & Target.Row) = "Python"
End Select
Next Target
'MsgBox wk.Name
Next wk
End Sub
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